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大学物理实验, 2024, 37(4): 37-42     https://doi.org/10.14139/i.cnki.cn22-1228.2024.04.007
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氯化钾溶液电化学阻抗测量过程中的等效电路模型研究
李敏言,袁朝庆,齐奕铭,祁园园,王俊涛*
河南工业大学 物理学院,河南 郑州 450001
Research on Equivalent Circuit Model in Electrochemical ImpedanceMeasurement of Potassium Chloride Solution
LI Minyan , YUAN Chaoqing,QI Yiming,Q Yuanyuan ,WANG Juntao*
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摘要 

等效电路模型是溶液电化学阻抗测量过程中研究其复杂物理化学过程的重要手段,在溶液电导率测量仪等设备的工程技术研发中具有重要的应用。 本文选取氯化钾溶液为研究对象,使用电化学工作站和铂黑平行双电极测量 0.01 mol/L至 1 mol/L 氯化钾溶液的阻抗谱,采用 Lima 和Randles 两种等效电路模型对测量结果进行拟合并对比两个模型的精度。 基于测量过程中不同频段下溶液的导电物理化学机制不同的事实,对测量结果进行分频段模拟以进一步提高模拟精度,并在  Lima 和 Randles 等效电路模型的基础上简化出高频等效电路模型。 采用高频等效电路模型对在高频下不不同浓度溶液的电导率测量结果进行模拟,对比并分析了浓度不同所引起的溶液内物理化学过程的差异。不同浓度溶液的电导率测量结果进行模拟,对比并分析了浓度不同所引起的溶液内物理化学过程的差异。

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李敏言
袁朝庆
齐奕铭
祁园园
王俊涛
关键词:  等效电路模型  氯化钾溶液  电化学阻抗谱  电导率     
Abstract: 

The equivalent cireuit model ( ECM)is an important means to study the complex physical andchemical process of the electrochemical impedance measurement of solution, and it has important application inthe engineering technology research and development of the equipment such as the solution conductivitymeasurement instrument,The potassium chloride solution ( KCl) was selected as the research object , and theimpedanee spectrum of 0.01 mol/l, to 1 mol/L, KCl was measured using electrochemical work station andplatinum black parallel double electrodes, The Lima and Randles ECM were used to fit the measurement resultsrespectively and the accuracy of the two models were compared. Based on the fact that the physical andchemical mechanism of the solution is diflerent at different AC excitation signal frequencies ,the measurementresults are simulated at high and low frequencies respectively, to further improve the simulation accuracy , andthe high-frequeney ECM is raised based on the Lima ECM and Randles ECM. High frequency ECM was used tosimulate the conductivity of KCl solution with different concentrations at high frequeney , and the differences of ohysical and chemical processes in solution caused by different coneentrations were compared and analyzed.

Key words:  the equivalent circuit model    potassium chloride solution    electrochemical impedance spectroscopy    electrical conductivity
               出版日期:  2024-08-25      发布日期:  2024-08-25      整期出版日期:  2024-08-25
ZTFLH:  O 64  
引用本文:    
李敏言, 袁朝庆, 齐奕铭, 祁园园, 王俊涛. 氯化钾溶液电化学阻抗测量过程中的等效电路模型研究 [J]. 大学物理实验, 2024, 37(4): 37-42.
LI Minyan , YUAN Chaoqing, QI Yiming, Q Yuanyuan , WANG Juntao. Research on Equivalent Circuit Model in Electrochemical ImpedanceMeasurement of Potassium Chloride Solution . Physical Experiment of College, 2024, 37(4): 37-42.
链接本文:  
http://dawushiyan.jlict.edu.cn/CN/10.14139/i.cnki.cn22-1228.2024.04.007  或          http://dawushiyan.jlict.edu.cn/CN/Y2024/V37/I4/37
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